Amino Acids

Amino Acid Side Chain Chemistry

Summary

The 20 standard amino acids are distinguished by their side chains (R groups), which determine protein structure, function, and interactions. Side chains vary in size, charge, hydrophobicity, and chemical reactivity, enabling the vast diversity of protein properties.

Key Points

  • 1Side chains determine protein structure, function, and interactions
  • 2Classified by polarity: nonpolar, polar, acidic, and basic
  • 3Ionization states depend on pKa and local environment
  • 4Key roles in catalysis, PTMs, and structural stabilization

The side chain is what makes each amino acid unique, providing the chemical diversity that enables proteins to perform their remarkable range of functions.

Classification of Side Chains

Nonpolar (Hydrophobic) Amino Acids

These residues tend to cluster in protein interiors:

#### Aliphatic Side Chains

- Glycine (Gly, G): H only; maximum conformational flexibility

- Alanine (Ala, A): -CH₃; small, hydrophobic

- Valine (Val, V): Branched -CH(CH₃)₂; β-branched

- Leucine (Leu, L): -CH₂CH(CH₃)₂; most common in proteins

- Isoleucine (Ile, I): β-branched, chiral at Cβ

#### Aromatic Side Chains

- Phenylalanine (Phe, F): Benzyl group; strongly hydrophobic

- Tryptophan (Trp, W): Indole ring; largest amino acid, UV absorbance at 280 nm

- Tyrosine (Tyr, Y): Hydroxyphenyl; can ionize (pKa ~10), phosphorylation site

#### Sulfur-Containing

- Methionine (Met, M): Thioether; initiator codon, oxidation-sensitive

- Cysteine (Cys, C): Thiol (-SH); forms disulfide bonds, highly reactive

#### Cyclic

- Proline (Pro, P): Pyrrolidine ring; restricts backbone, disrupts helices

Polar Uncharged Amino Acids

Capable of hydrogen bonding:

- Serine (Ser, S): -CH₂OH; phosphorylation site, nucleophile

- Threonine (Thr, T): -CH(OH)CH₃; β-branched, phosphorylation site

- Asparagine (Asn, N): -CH₂CONH₂; N-glycosylation site, deamidation-prone

- Glutamine (Gln, Q): -CH₂CH₂CONH₂; deamidation-prone

Charged Amino Acids

#### Positively Charged (Basic)

- Lysine (Lys, K): ε-amino group (pKa ~10.5); PTM sites (acetylation, methylation, ubiquitination)

- Arginine (Arg, R): Guanidinium group (pKa ~12.5); always charged at physiological pH

- Histidine (His, H): Imidazole (pKa ~6); protonation state changes near neutral pH, catalytic residue

#### Negatively Charged (Acidic)

- Aspartate (Asp, D): -CH₂COO⁻ (pKa ~3.9); metal coordination, catalysis

- Glutamate (Glu, E): -CH₂CH₂COO⁻ (pKa ~4.1); neurotransmitter precursor

Chemical Properties

Hydrophobicity Scales

Various scales quantify amino acid hydrophobicity:

- Kyte-Doolittle: Based on water-vapor transfer

- Eisenberg: Consensus scale

- Wimley-White: Interface and octanol scales

Hydrophobicity drives:

  • Protein folding (hydrophobic core)
  • Membrane protein topology
  • Protein-protein interactions
  • Ionization and pKa

    Side chain ionization affects protein function:

    | Residue | pKa (typical) |

    |---------|---------------|

    | Asp | 3.9 |

    | Glu | 4.1 |

    | His | 6.0 |

    | Cys | 8.3 |

    | Tyr | 10.1 |

    | Lys | 10.5 |

    | Arg | 12.5 |

    Note: Actual pKa values depend on local environment (can shift by several pH units).

    Reactivity

    #### Nucleophilic Side Chains

    Important in enzyme catalysis:

    - Serine: Serine proteases, esterases

    - Cysteine: Cysteine proteases, thiol chemistry

    - Histidine: Acid-base catalysis, metal coordination

    - Lysine: Schiff base formation

    #### Oxidation-Sensitive

    - Cysteine: Disulfides, sulfenic acid, sulfinic acid

    - Methionine: Methionine sulfoxide

    - Tryptophan: Various oxidation products

    - Tyrosine: Radical chemistry

    Functional Roles

    Enzyme Active Sites

    Catalytic residues often include:

    - Catalytic triad: Ser-His-Asp (serine proteases)

    - Metal coordination: His, Cys, Asp, Glu

    - Acid-base catalysis: His, Glu, Asp

    Post-Translational Modification Sites

    Side chains are targets for PTMs:

    - Phosphorylation: Ser, Thr, Tyr

    - Glycosylation: Asn (N-linked), Ser/Thr (O-linked)

    - Acetylation/Methylation: Lys

    - Ubiquitination: Lys

    Structural Roles

    - Salt bridges: Lys-Asp, Arg-Glu pairs

    - Disulfide bonds: Cys-Cys (stabilize tertiary/quaternary structure)

    - Aromatic stacking: Phe, Tyr, Trp π-π interactions

    - Cation-π interactions: Arg/Lys with aromatics

    Special Cases

    Selenocysteine (Sec, U)

    The "21st amino acid":

  • Selenium replaces sulfur
  • Encoded by UGA with special mRNA elements
  • Found in selenoproteins (glutathione peroxidase)
  • Pyrrolysine (Pyl, O)

    The "22nd amino acid":

  • Found in some methanogenic archaea
  • Encoded by UAG stop codon
  • Methylamine metabolism